High-frequency dielectric relaxation of liquid crystals: THz time-domain spectroscopy of liquid crystal colloids

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High-frequency dielectric relaxation of liquid crystals: THz time-domain spectroscopy of liquid crystal colloids

Please use this identifier to cite or link to this item: http://hdl.handle.net/10036/47367

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Title: High-frequency dielectric relaxation of liquid crystals: THz time-domain spectroscopy of liquid crystal colloids
Author: Oh-e, Masahito
Yokoyama, Hiroshi
Koeberg, Mattijs
Hendry, Euan
Bonn, Mischa
Citation: 14 (23), pp. 11433-11441
Publisher: Optical Society of America
Journal: Optics Express
Date Issued: 2006
URI: http://hdl.handle.net/10036/47367
DOI: 10.1364/OE.14.011433
Links: http://dx.doi.org/10.1364/OE.14.011433 http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-14-23-11433
Abstract: Terahertz time-domain spectroscopy has been used to study the dielectric relaxation of pure 4’–n-pentyl–4–cyanobiphenyl (5CB) liquid crystal (LC) and its mixtures with 10 µm SiO2 particles in the frequency range 0.2–2 THz. For the pure sample, we find that spatial inhomogeneities consisting of oriented domains, comparable in size to our probe area (~1 mm2), cause a large scatter in the measured dielectric function, due to varying contributions from the ordinary and extraordinary components. In the LC/particle mixtures, ordering of the LC at the surface of the SiO2 particles results in a break-up of these domains, giving rise to a spatially much more homogeneous dielectric response. The inferred dielectric function can be interpreted using effective medium theory and the Debye relaxation model. We observe this stabilizing effect for interparticle distances < ~30 µm, setting a lower limit for the size of oriented domains in the bulk LC.
Type: Article
Description: Copyright © 2006 Optical Society of America. This paper was published in Optics Express and is made available as an electronic reprint with the permission of OSA. The paper can be found at the following URL on the OSA website: http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-14-23-11433 . Systematic or multiple reproduction or distribution to multiple locations via electronic or other means is prohibited and is subject to penalties under law.
ISSN: 1094-4087


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