Retrieving the susceptibility from time-resolved terahertz experiments

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Retrieving the susceptibility from time-resolved terahertz experiments

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Title: Retrieving the susceptibility from time-resolved terahertz experiments
Author: Schins, Juleon M.
Hendry, Euan
Bonn, Mischa
Muller, H. G.
Citation: 127 (9), article 094308
Publisher: American Institute of Physics
Journal: Journal of Chemical Physics
Date Issued: 2007
DOI: 10.1063/1.2761915
Abstract: We present an analytical expression for the observed signal in time- and phase-resolved pump-probe studies, with particular emphasis on terahertz time-domain spectroscopy. Maxwell's equations are solved for the response of damped, harmonic oscillators to a driving probe field in the perturbative regime. Our analytical expressions agree with the one previously reported in the literature [Nemec et al., J. Chem. Phys. 122, 104503 (2005)] in the Drude limit; however, they differ in the case of a vibrational resonance
Type: Article
Description: Copyright © 2007 American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics. The following article appeared in Journal of Chemical Physics 127 (2007) and may be found at
Keywords: harmonic oscillatorslaser beamsMaxwell equationsmeasurement by laser beamsubmillimetre wave spectratime resolved spectra
ISSN: 0021-9606

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