Microscopic theory of exciton and trion polaritons in doped monolayers of transition metal dichalcogenides
| dc.contributor.author | Zhumagulov, YV | |
| dc.contributor.author | Chiavazzo, S | |
| dc.contributor.author | Gulevich, DR | |
| dc.contributor.author | Perebeinos, V | |
| dc.contributor.author | Shelykh, IA | |
| dc.contributor.author | Kyriienko, O | |
| dc.date.accessioned | 2022-05-06T12:22:28Z | |
| dc.date.issued | 2022-04-28 | |
| dc.date.updated | 2022-05-06T10:52:33Z | |
| dc.description.abstract | We study a doped transition metal dichalcogenide (TMDC) monolayer in an optical microcavity. Using the microscopic theory, we simulate spectra of quasiparticles emerging due to the interaction of material excitations and a high-finesse optical mode, providing a comprehensive analysis of optical spectra as a function of Fermi energy and predicting several modes in the strong light-matter coupling regime. In addition to exciton-polaritons and trion-polaritons, we report polaritonic modes that become bright due to the interaction of excitons with free carriers. At large doping, we reveal strongly coupled modes corresponding to excited trions that hybridize with a cavity mode. We also demonstrate that the increase of carrier concentration can change the nature of the system’s ground state from the dark to the bright one. Our results offer a unified description of polaritonic modes in a wide range of free electron densities. | en_GB |
| dc.description.sponsorship | Deutsche Forschungsgemeinschaft (DFG) | en_GB |
| dc.description.sponsorship | Russian Science Foundation | en_GB |
| dc.description.sponsorship | Icelandic Research Fund | en_GB |
| dc.description.sponsorship | Russian Foundation for Basic Research (RFBR) | en_GB |
| dc.description.sponsorship | Engineering and Physical Sciences Research Council (EPSRC) | en_GB |
| dc.description.sponsorship | University at Buffalo | en_GB |
| dc.description.sponsorship | SUNY Research Seed Grant Program | en_GB |
| dc.identifier.citation | Vol. 8, article 92 | en_GB |
| dc.identifier.doi | https://doi.org/10.1038/s41524-022-00775-x | |
| dc.identifier.grantnumber | 443416183 | en_GB |
| dc.identifier.grantnumber | 20-12-00224 | en_GB |
| dc.identifier.grantnumber | 21-52-12038 | en_GB |
| dc.identifier.grantnumber | EP/V00171X/1 | en_GB |
| dc.identifier.uri | http://hdl.handle.net/10871/129535 | |
| dc.identifier | ORCID: 0000-0002-6259-6570 (Kyriienko, Oleksandr) | |
| dc.language.iso | en | en_GB |
| dc.publisher | Nature Research | en_GB |
| dc.rights | © The Author(s) 2022. Open Access. This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. | en_GB |
| dc.title | Microscopic theory of exciton and trion polaritons in doped monolayers of transition metal dichalcogenides | en_GB |
| dc.type | Article | en_GB |
| dc.date.available | 2022-05-06T12:22:28Z | |
| dc.identifier.issn | 2057-3960 | |
| dc.description | This is the final version. Available on open access from Nature Research via the DOI in this record | en_GB |
| dc.description | Data availability: The data that support the findings of this study are available from the corresponding author upon reasonable request. | en_GB |
| dc.description | Code availability: All the codes were implemented using home-built programs, which use standard open-source software packages. | en_GB |
| dc.identifier.journal | npj Computational Materials | en_GB |
| dc.relation.ispartof | npj Computational Materials | |
| dc.rights.uri | https://creativecommons.org/licenses/by/4.0/ | en_GB |
| dcterms.dateAccepted | 2022-03-29 | |
| rioxxterms.version | VoR | en_GB |
| rioxxterms.licenseref.startdate | 2022-04-28 | |
| rioxxterms.type | Journal Article/Review | en_GB |
| refterms.dateFCD | 2022-05-06T10:52:43Z | |
| refterms.versionFCD | AM | |
| refterms.dateFOA | 2022-05-06T12:22:34Z | |
| refterms.panel | B | en_GB |
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